Closed‐Loop Recyclable and Extrusion Reprocessable Thermosets Enabled by Guanylthiourea Structure
2024

Recyclable Thermosets from Guanylthiourea Structure

publication Evidence: high

Author Information

Author(s): Yu Zhen, Liu Yanlin, Zhou Xiangyu, Fang Yajin, Tang Zhaobin, Zhu Jin, Zhang Junping

Primary Institution: Lanzhou Institute of Chemical Physics, Chinese Academy of Sciences

Hypothesis

Can a thermoset network based on guanythiourea structure be effectively recycled through various methods?

Conclusion

The GTUH network demonstrates exceptional performance and rapid reprocessing capabilities, enabling effective recycling and restoration of mechanical properties.

Supporting Evidence

  • The GTUH network can be recycled through continuous extrusion processing due to multiple reversible mechanisms.
  • Mechanical properties of the recycled network can be maintained or improved after reprocessing.
  • Research indicates promising potential applications for this material in the circular economy.

Takeaway

This study shows how a special type of plastic can be recycled easily and reused, making it better for the environment.

Methodology

The GTUH network was synthesized via nucleophilic addition reaction and evaluated for its recycling capabilities through various processing methods.

Limitations

Challenges persist in maintaining performance metrics such as glass transition temperature and dimensional stability.

Digital Object Identifier (DOI)

10.1002/advs.202410773

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