Electron Capture Dissociation, Electron Detachment Dissociation, and Collision-Induced Dissociation of Polyamidoamine (PAMAM) Dendrimer Ions with Amino, Amidoethanol, and Sodium Carboxylate Surface Groups
2008

Study of PAMAM Dendrimers and Their Dissociation

publication Evidence: moderate

Author Information

Author(s): Malgorzata A. Kaczorowska, Helen J. Cooper

Primary Institution: School of Biosciences, University of Birmingham

Hypothesis

The study investigates how the structure and surface groups of PAMAM dendrimers affect their electron-mediated dissociation.

Conclusion

The results indicate that electron-mediated dissociation of PAMAM dendrimers is independent of the surface group nature and occurs mainly in the innermost generations, while collision-induced dissociation is dependent on the surface group and occurs in the outermost generation.

Supporting Evidence

  • ECD and EDD produced simpler mass spectra compared to CID.
  • Fragmentation in ECD and EDD was dominated by cleavage at tertiary amines.
  • CID showed a strong dependence on the nature of the surface groups.

Takeaway

This study looks at how different types of PAMAM dendrimers break apart when hit by electrons, finding that the way they break doesn't change much based on their surface features.

Methodology

The study used mass spectrometry techniques including ECD, EDD, and CID to analyze PAMAM dendrimers.

Digital Object Identifier (DOI)

10.1016/j.jasms.2008.06.016

Want to read the original?

Access the complete publication on the publisher's website

View Original Publication