Robust proteome profiling of cysteine-reactive fragments using label-free chemoproteomics
2024

New Method for Profiling Cysteine-Reacting Fragments in Proteomics

Sample size: 80 publication 10 minutes Evidence: high

Author Information

Author(s): George S. Biggs, Emma E. Cawood, Aini Vuorinen, William J. McCarthy, Harry Wilders, Ioannis G. Riziotis, Antonie J. van der Zouwen, Jonathan Pettinger, Luke Nightingale, Peiling Chen, Andrew J. Powell, David House, Simon J. Boulton, J. Mark Skehel, Katrin Rittinger, Jacob T. Bush

Primary Institution: The Francis Crick Institute, London, UK

Hypothesis

Can a high-throughput, label-free chemoproteomics platform effectively identify ligand-protein interactions across the human proteome?

Conclusion

The study successfully developed a high-throughput platform that identified over 400 ligand-protein interactions using cysteine-reactive fragments.

Supporting Evidence

  • The platform identified >400 ligand-protein interactions from 80 screened fragments.
  • Data completeness was high, with two-thirds of peptides detected in ≥75% of samples.
  • Over 8000 proteins were detected, representing ~40% of the human proteome.

Takeaway

Researchers created a new way to find how small molecules interact with proteins in our bodies, which can help in making new medicines.

Methodology

The study used a label-free quantification proteomics platform to profile cysteine-reactive fragments against the native proteome, employing data-independent acquisition for high-throughput screening.

Limitations

The platform achieves ~40% coverage of the proteome but less than 15% of the entire cysteinome.

Statistical Information

P-Value

p<0.05

Statistical Significance

p<0.05

Digital Object Identifier (DOI)

10.1038/s41467-024-55057-5

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